Harrop, who arrived in Somerset in July 2015, will leave the Academy to pursue a new venture elsewhere.
Having played an integral role in building a successful category three youth setup, Chairman of the Academy Andy Rossiter thanked Harrop for his efforts.
“We wish to extend our thanks to Geoff for the hard work and commitment he has put in since arriving at the Club.
“He has played a big part in moving forward the Academy since its inception and we wish him all the best in his next chapter.”
Yeovil Town Academy are undertaking the necessary recruitment processes to find a successor, and everyone at Yeovil Town Football Club extend their thanks to Geoff for helping to build an Academy which will bear fruits in the future.